Quantum-Enhanced Nonlinear Spectroscopy

Frank Schlawin (Autor)

Buch | Softcover

XIV, 259 Seiten

2018 | 1. Softcover reprint of the original 1st ed. 2017
Springer International Publishing (Verlag)
978-3-319-83049-0 (ISBN)

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This thesis focuses on nonlinear spectroscopy from a quantum optics perspective. First, it provides a detailed introduction to nonlinear optical signals; starting from Glauber's photon counting formalism, it establishes the diagrammatic formulation, which forms the backbone of nonlinear molecular spectroscopy. The main body of the thesis investigates the impact of quantum correlations in entangled photon states on two-photon transitions, with a particular focus on the time-energy uncertainty, which restricts the possible simultaneous time and frequency resolution in measurements. It found that this can be violated with entangled light for individual transitions. The thesis then presents simulations of possible experimental setups that could exploit this quantum advantage. The final chapter is devoted to an application of the rapidly growing field of multidimensional spectroscopy to trapped ion chains, where it is employed to investigate nonequilibrium properties in quantum simulations.

Introduction.- Background.- Nonlinear Optical Signals.- Excited State Distributions and Fluorescence Signals.- Pump-Probe Measurements with Entangled Photons.- Interferometric Setups.- Frequency Conversion.- Trapped Ion Spectroscopy.- Conclusions and Outlook.

Erscheinungsdatum	05.03.2022
Reihe/Serie	Springer Theses
Zusatzinfo	XIV, 259 p. 95 illus., 14 illus. in color.
Verlagsort	Cham
Sprache	englisch
Maße	155 x 235 mm
Gewicht	427 g
Themenwelt	Naturwissenschaften ► Chemie ► Analytische Chemie
	Naturwissenschaften ► Physik / Astronomie ► Optik
	Naturwissenschaften ► Physik / Astronomie ► Quantenphysik
	Naturwissenschaften ► Physik / Astronomie ► Theoretische Physik
Schlagworte	Entangled Photon States • Glauber's Formalism • Multidimensional Spectroscopy • Nonlinear molecular spectroscopy • Nonlinear Quantum Optics • Quantum advantage in spectroscopy • Quantum Enhancement • Trapped Ion Spectroscopy
ISBN-10	3-319-83049-X / 331983049X
ISBN-13	978-3-319-83049-0 / 9783319830490
Zustand	Neuware